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Abstract Cuprous oxide ($$\hbox {Cu}{}_2\hbox {O}$$ $\text{Cu}{}_2\text{O}$) has recently emerged as a promising material in solid-state quantum technology, specifically for its excitonic Rydberg states characterized by large principal quantum numbers (n). The significant wavefunction size of these highly-excited states (proportional to$$n^2$$ $n^2$) enables strong long-range dipole-dipole (proportional to$$n^4$$ $n^4$) and van der Waals interactions (proportional to$$n^{11}$$ $n^{11}$). Currently, the highest-lying Rydberg states are found in naturally occurring$$\hbox {Cu}_2\hbox {O}$$ ${\text{Cu}}_2\text{O}$. However, for technological applications, the ability to grow high-quality synthetic samples is essential. The fabrication of thin-film$$\hbox {Cu}{}_2\hbox {O}$$ $\text{Cu}{}_2\text{O}$samples is of particular interest as they hold potential for observing extreme single-photon nonlinearities through the Rydberg blockade. Nevertheless, due to the susceptibility of high-lying states to charged impurities, growing synthetic samples of sufficient quality poses a substantial challenge. This study successfully demonstrates the CMOS-compatible synthesis of a$$\hbox {Cu}{}_2\hbox {O}$$ $\text{Cu}{}_2\text{O}$thin film on a transparent substrate that showcases Rydberg excitons up to$$n = 8$$ $n=8$which is readily suitable for photonic device fabrications. These findings mark a significant advancement towards the realization of scalable and on-chip integrable Rydberg quantum technologies. 

We demonstrate the integration of superconducting single-photon detectors onto arbitrary photonic substrates via transfer printing. Using this method, we show single-photon detection in a lithium niobate on insulator photonic circuit. 

Abstract Quantum technologies are poised to move the foundational principles of quantum physics to the forefront of applications. This roadmap identifies some of the key challenges and provides insights on material innovations underlying a range of exciting quantum technology frontiers. Over the past decades, hardware platforms enabling different quantum technologies have reached varying levels of maturity. This has allowed for first proof-of-principle demonstrations of quantum supremacy, for example quantum computers surpassing their classical counterparts, quantum communication with reliable security guaranteed by laws of quantum mechanics, and quantum sensors uniting the advantages of high sensitivity, high spatial resolution, and small footprints. In all cases, however, advancing these technologies to the next level of applications in relevant environments requires further development and innovations in the underlying materials. From a wealth of hardware platforms, we select representative and promising material systems in currently investigated quantum technologies. These include both the inherent quantum bit systems and materials playing supportive or enabling roles, and cover trapped ions, neutral atom arrays, rare earth ion systems, donors in silicon, color centers and defects in wide-band gap materials, two-dimensional materials and superconducting materials for single-photon detectors. Advancing these materials frontiers will require innovations from a diverse community of scientific expertise, and hence this roadmap will be of interest to a broad spectrum of disciplines.